A great movie must incorporate a great script and for a great script you need unforgettable lines.

"The board is set, the pieces are moving" (Ian Mckellen, The Lord of the Rings The Return of the King)

"Winter must be cold for those with no warm memories...and we've already missed the spring" (Deborah Kerr, An Affair to Remember)

"Sell crazy someplace else, we're all stocked up here." (Jack Nicholson, As Good As It Gets)

"Obi-Wan... Now, thats a name I haven't heard in a long time." (Alec Guinness, Star Wars)

But mostly a great line depends on the way its delivered.

"Look it's not in my nature to be mysterious, but I can't talk about it and I can't talk about why." (Brad Pitt, Ocean's Twelve)

"We can do this with or without violence, it's up to you." (Holly Hunter, A Life Less Ordinary)

(While being chased by a T-Rex) "Must go faster." (Jeff Goldblum, Jurassic Park)

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